期刊
ACS APPLIED POLYMER MATERIALS
卷 2, 期 3, 页码 1304-1311出版社
AMER CHEMICAL SOC
DOI: 10.1021/acsapm.9b01189
关键词
Heterogeneity; Self-potential; Surface charge patchiness; Fluid interface; Optical tweezers
资金
- National Research Foundation (NRF) of Korea [NRF-2014R1A5A1009799, NRF-2017R1A2B4003123, NRF-2016R1D1A1B03932999, NRF-2019R1C1C1009427]
Electrostatic self-potentials of individual particles trapped at an oil-water interface were determined, and the effects of surface chemical nonuniformity on heterogeneous self-potentials and equilibrium microstructures were investigated. Direct measurement of the pair interactions and the self-potentials of polystyrene microspheres were performed using optical laser tweezers. The individual particles had different self-potentials even when they possessed the same surface functionalities. Atomic force microscopy measurements elucidated the relationship between nonuniform surface charge distribution and heterogeneity and magnitude of self-potentials. Monte Carlo simulations demonstrated that self-potential heterogeneity led to the formation of more melted microstructures that showed excellent consistency with experiments.
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