期刊
MATTER
卷 2, 期 1, 页码 111-118出版社
ELSEVIER
DOI: 10.1016/j.matt.2019.08.001
关键词
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资金
- National Natural Science Foundation of China [11674148, 11334003, 11704177]
- Guangdong Natural Science Funds for Distinguished Young Scholars [2017B030306008]
- General Research Fund [17304318]
- Collaborative Research Fund from the Research Grant Council [C7036-17W]
- Hong Kong Special Administrative Region
- Center for Computational Science and Engineering of Southern University of Science and Technology
Two-dimensional (2D) non-covalent and covalent networks are interesting because their tailorable architectures offer fresh applications in sensing, catalysis, gas storage, and topological structures. So far, rational design of these networks has been explored exclusively involving organic molecules based on the concept of modular assembly. Here, we demonstrate that, by using molecular-beam epitaxy, we can isolate inorganic blocks to form a 2D porous gold-phosphorus network (AuPhoN), wherein blue phosphorene (blueP) subunits are linked by gold atoms on an Au surface. We provide evidence that such metal-phosphorus networks are tunable in their chemical functionalities and electronic properties by simply altering the linkers and subunits. Our work provides insights to tailor low-dimension architectures of inorganic networks that maintain good long-range order and are stable over a wide temperature range.
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