期刊
PHYSICAL REVIEW LETTERS
卷 84, 期 13, 页码 2881-2884出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.84.2881
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The three sire-sire partial structure factors for water have been measured as a function of pressure, using neutron diffraction, at a temperature of 268 K. It is found that the measured structure functions imply a continuous transformation with increasing pressure from a low-density form of water (rho(L) similar to 0.0295 molecules/Angstrom(3)), with an open, hydrogen-bonded tetrahedral structure, to a high-density form of water (rho(H) similar to 0.0402 molecules/Angstrom(3)), with nontetrahedral O-O-O angles and a collapsed second coordination shell, which implies broken hydrogen bonds between the first and second coordination shells.
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