期刊
BIOMATERIALS
卷 32, 期 21, 页码 4877-4884出版社
ELSEVIER SCI LTD
DOI: 10.1016/j.biomaterials.2011.03.029
关键词
Single particle SERS; Polyhedral Ag mesocages; Biosensor; Ag2O template
资金
- Alexander-von-Humboldt Foundation
- 'Xi'an Jiaotong University
- Fundamental Research Funds for the Central Universities [08142008]
- National Natural Science Foundation of China [50901056, 5107116, 60736041, 10874238]
Surface-enhanced Raman scattering-based signal detection and molecular identification faces the lack of reproducibility and reliability thus hampers its practical applications. Here, we demonstrate a facile particle mediated aggregation protocol to synthesize highly roughened mesosuperstructure - silver polyhedral mesocages. The individual silver octahedral mesocage, owing to highly-roughed surface topography, anisotropic growth as well as intraparticle effect, creates homogenously distributed multiple effective hot spots on the surface of single mesoparticle, hereby exhibits a high reproducibility and an unusual SERS enhancement, i.e., similar to 10(8)-10(9) magnitude. As such, the current protocol opens avenues for the fabrication of structurally reproducible mesosuperstructure-based SERS sensors. (C) 2011 Elsevier Ltd. All rights reserved.
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