期刊
JOURNAL OF MAGNETISM AND MAGNETIC MATERIALS
卷 213, 期 1-2, 页码 135-142出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/S0304-8853(99)00541-7
关键词
disorder; binomial distribution; alloys; Mossbauer; hyperfine field
In order to give an interpretation of the room temperature hyperfine magnetic field distributions of disordered Fe0.9-xMn0.1Alx (0.1 less than or equal to x less than or equal to 0.5) alloys, we employ a local model based on a binomial distribution method. In the model, the constituent atoms are assumed to be randomly distributed in a BCC lattice accordingly with the disordered character of the system and its crystalline structure. Results show that the substitution of an iron atom by an aluminum atom, in the first Fe coordination shell, produces a reduction in the hyperfine field of 20.8 kOe. Analogously, the substitution of Fe by Mn produces a reduction of 24.1 kOe. Differently from this, substitutions in the second coordination shell produce reductions of 6.6 and 3.3 kOe for Al and Mn, respectively. The model also allows to obtain the average hyperfine field as well as to determine the most probable configurations (sites) of the system, involving nearest and next nearest neighbors. Finally, results are compared with experimental results obtained by Mossbauer spectroscopy. (C) 2000 Elsevier Science B.V. All rights reserved.
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