期刊
PHYSICAL REVIEW LETTERS
卷 84, 期 21, 页码 4862-4865出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.84.4862
关键词
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The effective charge of a rigid polyelectrolyte (PE) approaching an oppositely charged surface is studied. The eases of a weak (annealed) and strongly charged PE with condensed counterions (such as DNA) are discussed. In the most interesting case of the adsorption onto a substrate of low dielectric constant (such as a lipid membrane or a mica sheet) the condensed counterions are and always released as the PE approaches the substrate, because of the major importance of the image-charge effect. For the adsorption onto a surface with freely moving charges, the image-charge effect becomes less important and full release is often expected.
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