期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 122, 期 28, 页码 6624-6628出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja000930i
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Enantioselective total syntheses of the antitumor alkaloids. (+)-narciclasine and (+)-pancratistatin, are reported. These syntheses feature a stereo- and regiocontrolled aryl enamide photocyclization to construct a common, advanced intermediate possessing a trans-fused BC substructure. Differential functional group interchange in the C-ring of this phenanthridone core structure allows for the production of the two target natural products in enantiomerically pure form.
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