期刊
ASTROPHYSICAL JOURNAL
卷 543, 期 2, 页码 764-774出版社
UNIV CHICAGO PRESS
DOI: 10.1086/317137
关键词
ISM : molecules; methods : laboratory; molecular data; molecular processes
We present an experimental study of the dissociative recombination (DR) of H3O+ and its isotopomers D3O+ and HD2O+ performed at the ASTRID storage ring. DR cross sections have been measured as a function of energy, while complete branching ratios have been measured at E = 0. The H3O+ data yield an accurate determination of the branching ratio for water formation (0.25 +/- 0.01). The three molecular ions-H3O+, D3O+, and HD2O+-show a marked resemblance concerning cross sections and branching ratios. The only observed isotope effect is in the fragmentation pattern of HD2O+, where the release of a light fragment is favored over release of a heavier fragment. As a consequence, an enhanced production of deuterated molecules takes place as a result of the DR process.
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