期刊
JOURNAL OF PHYSICAL CHEMISTRY A
卷 106, 期 3, 页码 453-457出版社
AMER CHEMICAL SOC
DOI: 10.1021/jp012986k
关键词
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The vibrational OH-stretch spectra of size-selected pure water (H(2)O)(9) clusters, measured at two different temperatures, have been used to identify isomeric transitions. The broad, featureless high-temperature, liquid-like spectrum resembles that of water, while the structured low- temperature, solid-like spectrum differs appreciably from that of ice. Accompanying calculations suggest that the low-temperature spectra originate from two cube-like structures. The high-temperature spectra appear to be above an isomeric transition to more open amorphous arrangements of fused three- to five-membered rings.
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