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Circular dichroism in K-shell ionization from fixed-in-space CO and N2 molecules -: art. no. 073002

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PHYSICAL REVIEW LETTERS
卷 88, 期 7, 页码 -

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AMERICAN PHYSICAL SOC
DOI: 10.1103/PhysRevLett.88.073002

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We have measured the angular distributions of 1s photoelectrons excited by circularly and linearly polarized light from fixed-in-space CO and N-2 molecules, in the vicinity of their shape resonances. A strong circular dichroism, i.e., a strong dependence on the sense of rotation of the polarization vector of the photons, is found for both molecules. State-of-the-art one-electron multiple scattering and partially correlated random phase approximation calculations are in good agreement with many, but not all, aspects of the experimental data.

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