期刊
CHEMICAL PHYSICS LETTERS
卷 354, 期 5-6, 页码 367-375出版社
ELSEVIER
DOI: 10.1016/S0009-2614(02)00141-0
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An accurate instrumental response function is needed to deconvolute fluorescence data obtained by time-correlated single-photon counting (TCSPC) upon multi-photon excitation. Hitherto the response function was obtained by measuring Rayleigh scattering (RS) from colloidal solutions, as is also used in one-photon excited fluorescence. We show that hyper Rayleigh scattering (HRS) provides a better choice for deconvolution of fluorescence decays, as obtained by TCSPC and two-photon excitation (TPE). The one- and two-photon response functions were monitored as RS and HRS from colloidal gold particles at 800 and 400 nm, respectively. (C) 2002 Published by Elsevier Science B.V.
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