期刊
JOURNAL OF PHYSICAL CHEMISTRY B
卷 106, 期 33, 页码 8313-8317出版社
AMER CHEMICAL SOC
DOI: 10.1021/jp0208440
关键词
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Simple closed-form expressions of line-shape functions are derived for models of a two-level chromophore linearly coupled to harmonic oscillator baths on the basis of an accurate approximation for the coth(x/2) function. The expressions are valid for arbitrary temperature and can be extended to a general spectral density given by a sum of algebraic terms with exponential damping factors. Detailed analyses for three typical spectral densities reveal, in the strong-coupling limit, general temperature dependences of the line widths, and in the weak coupling limit, important features of temperature dependence.
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