期刊
JOURNAL OF NONLINEAR OPTICAL PHYSICS & MATERIALS
卷 11, 期 4, 页码 421-432出版社
WORLD SCIENTIFIC PUBL CO PTE LTD
DOI: 10.1142/S0218863502001103
关键词
nonlinear optics; second-harmonic generation; metal nanoparticles; nanostructures
The optical properties of nanoscopic arrays of metal particles are dominated by plasmon resonances and electromagnetic interaction between the particles. We use electron-beam lithography to prepare arrays of noncentrosymmetric gold particles and study their linear and second-order nonlinear optical properties. By varying the orientation of the particles in a fixed lattice, we observe shifts in the polarized linear extinction spectra. The second-harmonic generation efficiencies of the two types of samples differ by up to 60%. The results show that the properties of the samples are sensitive to the smallest details of their structure.
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