期刊
PHYSICAL REVIEW LETTERS
卷 90, 期 4, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.90.047402
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Coherent nuclear motion of the carbon backbone is monitored in real time in substituted poly(phenylene)-vinylene in both excited and ground electronic state using sub-10-fs light pulses. Characteristic features of the intrachain vibrational dynamics are obtained. We observe vibrational dephasing in the excited state within 1 ps (time constant T(2e)approximate to300 fs). These findings are in agreement with the molecular picture for photoexcitation in conjugated polymers.
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