期刊
JOURNAL OF PHYSICAL CHEMISTRY A
卷 107, 期 7, 页码 956-961出版社
AMER CHEMICAL SOC
DOI: 10.1021/jp027134e
关键词
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The condensed-phase solvation dynamics of those molecules in immediate proximity to an excited-state chromophore were probed with femtosecond time resolution by a technique that employs resonant optical excitation of the chromophore followed by a nonresonant third-order Raman probe of the solvent. This new method provides a microscopic perspective from the point of view of those solvent molecules that make up the local environment of a dynamic event. In this initial study, we have investigated the solvation dynamics of 9,10-diphenylanthracene dissolved in chloroform.
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