期刊
CHEMICAL PHYSICS LETTERS
卷 369, 期 5-6, 页码 525-533出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/S0009-2614(02)02030-4
关键词
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Optimal control theory is used to design laser pulses that enhance the trans-cis photoisomerization of retinal, which is modeled by coupled potential curves to examine coupling effects on control mechanisms. Based on numerical results, a new type of pump-dump control pathway, in which an optimal pulse achieves high target probability without directly modifying a potential coupling, is proposed. The key feature of this control is that a shaped wave packet passes a curve-crossing point adiabatically in the ground electronic state. (C) 2003 Elsevier Science B.V. All rights reserved.
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