期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 125, 期 14, 页码 4240-4252出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja021380m
关键词
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Hinckdentine A is an alkaloid isolated from the bryozoan Hincksinoflustra denticulate. This natural product contains a novel and unique 11b,12,13,14,15,16-hexahydroazepino[4',5':2,3]indolo[1,2-c]quinazoline ring system that has not previously been synthesized. We have synthesized 8-desbromohinckdentine A from a 2-aryl indole by first preparing the quaternary center of the natural product and then building the seven-membered lactam and dihydropyrimidine rings onto this intermediate to form the framework of hinckdentine A.
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