期刊
JOURNAL OF NON-CRYSTALLINE SOLIDS
卷 326, 期 -, 页码 379-384出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/S0022-3093(03)00441-1
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Floppy modes and relaxation processes in the GexSe1-x glasses system are studied by vibrational methods. We reporL Raman spectral line shapes over a temperature range from 100 to 300 K. Normalized frequency shifts with temperature of the GeSe4/2 breathing mode and the Se-Se stretching mode depend on the Ge composition. The results are associated with the stiffness transition window in which we suggest a radical decrease of Se-n (n > 2) segments which could be regarded as the microscopic origin of floppy modes in the Se-containing network glasses. (C) 2003 Published by Elsevier B.V.
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