Phase-matched four-wave mixing in higher-order modes of microstructure fibers allows unprecedentedly high efficiencies of anti-Stokes frequency conversion to be achieved for subnanojoule famtosecond laser pulses. 70-fs pulses of 790-nm radiation were used to generate an anti-Stokes component at 520-530 nm in a higher-order mode of a microstructure fiber With a 4.8-mum core. The maximum ratio of the anti-Stokes signal energy to the energy of the pump component in the output spectrum is estimated as 1.7. (C) 2003 Optical Society of America.
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