期刊
JOURNAL OF PHYSICAL CHEMISTRY A
卷 107, 期 46, 页码 9937-9945出版社
AMER CHEMICAL SOC
DOI: 10.1021/jp030708a
关键词
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This paper explores the benefit of using time dependent basis sets in the description of adiabatic population transfer between molecular states. Using a time dependent basis set formalism, we develop a counter-diabatic field paradigm that generates adiabatic population transfer for apparently unfavorable conditions. We also describe a time dependent perturbation approach to account for the effect of stochastic dephasing on adiabatic population transfer.
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