Pure rotational coherent anti-Stokes Raman spectroscopy is applied for quantitative gas-phase temperature measurements in the vaporizing spray of an automotive fuel injector. Interferences from elastically scattered stray light are greatly reduced by use of a polarization technique and spectral filtering in a double monochromator. The applicability of this technique to probing low-temperature sprays is successfully demonstrated. (C) 2004 Optical Society of America.
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