期刊
PHYSICAL REVIEW LETTERS
卷 92, 期 21, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.92.218301
关键词
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The theory of Forster resonance energy transfer is generalized for multichromophoric (MC) and nonequilibrium situations. For the first time, it is clarified that the far-field linear spectroscopic information is insufficient for the determination of the reaction rate and that distance dependence of the rate can vary with the disorder and temperature. Application to a light harvesting complex LH2 reveals the important consequences of a MC structure.
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