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Multichromophoric Forster resonance energy transfer

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PHYSICAL REVIEW LETTERS
卷 92, 期 21, 页码 -

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AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.92.218301

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The theory of Forster resonance energy transfer is generalized for multichromophoric (MC) and nonequilibrium situations. For the first time, it is clarified that the far-field linear spectroscopic information is insufficient for the determination of the reaction rate and that distance dependence of the rate can vary with the disorder and temperature. Application to a light harvesting complex LH2 reveals the important consequences of a MC structure.

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