期刊
JOURNAL OF APPLIED PHYSICS
卷 95, 期 11, 页码 6675-6677出版社
AMER INST PHYSICS
DOI: 10.1063/1.1667834
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We present the consistent electronic and magnetic properties in high-quality defect-controlled single crystals of CaB6, based on temperature-dependent transport and isothermal magnetization. Pure CaB6 single crystals, synthesized with 99.9999%-pure boron, exhibited fully semiconducting characteristics, such as monotonic resistance for 2-300 K. Boron-related defects formed in CaB6 single crystals, synthesized with 99.9%-pure boron, induced extra free charge carriers. Remarkably, no ferromagnetic signals were detected from single crystals made with 99.9999%-pure boron, regardless of stoichiometry, whereas those made with 99.9%-boron exhibited ferromagnetism within a finite range of carrier density. This indicates that the boron-related defects generate both the local magnetic moments associated with the exotic ferromagnetism and extra free charge carriers. (C) 2004 American Institute of Physics.
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