期刊
PHYSICAL REVIEW LETTERS
卷 93, 期 4, 页码 -出版社
AMER PHYSICAL SOC
DOI: 10.1103/PhysRevLett.93.048301
关键词
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Dynamics following electron photodetachment in a complex of a chloride anion with ammonia is explored by a combination of electronic structure and quantum dynamical methods. This system serves as a prototype for investigating a hitherto unexplored class of chemical reactions-nonadiabatic proton transfer triggered by a detachment of an electron. All the reactive and nonreactive channels of this process are characterized and the respective quantum yields are presented.
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