期刊
APPLIED SURFACE SCIENCE
卷 255, 期 24, 页码 9712-9716出版社
ELSEVIER SCIENCE BV
DOI: 10.1016/j.apsusc.2009.04.139
关键词
Femtosecond laser ablation; Pump-probe; Optics of hot Al and Au
The theory and experiments concerned with the electron-ion thermal relaxation and melting of overheated crystal lattice constitute the subject of this paper. The physical model includes two-temperature (2T) equation of state, many-body interatomic potential, the electron-ion energy exchange, electron thermal conductivity, and optical properties of solid, liquid, and two phase solid-liquid mixture. Two-temperature hydrodynamics and molecular dynamics codes are used. An experimental setup with pump-probe technique is used to follow evolution of an irradiated target with a short time step 100 fs between the probe femtosecond laser pulses. Accuracy of measurements of reflection coefficient and phase of reflected probe light are 1% and similar to 1 nm, respectively. It is found that, firstly, the electron-electron collisions make a minor contribution to a light absorption in solid Al at moderate intensities; secondly, the phase shift of a reflected probe results from heating of ion subsystem and kinetics of melting of Al crystal during 0 ps < t < 4 ps, where t is time delay between the pump and probe pulses measured from the maximum of the pump; thirdly, the optical response of Au to a pump shows a marked contrast to that of Al on account of excitation of d-electrons. (C) 2009 Elsevier B.V. All rights reserved.
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