期刊
APPLIED PHYSICS LETTERS
卷 104, 期 21, 页码 -出版社
AMER INST PHYSICS
DOI: 10.1063/1.4880899
关键词
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资金
- U.S. Department of Energy/National Renewable Energy Laboratory's Laboratory Directed Research and Development (LDRD) program [DE-AC36-08GO28308]
We report an 11.4%-efficient perovskite CH3NH3PbI3 solar cell using low-cost molybdenum oxide/aluminum (i.e., MoOx/Al) as an alternative top contact to replace noble/precious metals (e. g., Au or Ag) for extracting photogenerated holes. The device performance of perovskite solar cells using a MoOx/Al top contact is comparable to that of cells using the standard Ag top contact. Analysis of impedance spectroscopy measurements suggests that using 10-nm-thick MoOx and Al does not affect charge-recombination properties of perovskite solar cells. Using a thicker (20-nm) MoOx layer leads to a lower cell performance caused mainly by a reduced fill factor. Our results suggest that MoOx/Al is promising as a low-cost and effective hole-extraction contact for perovskite solar cells.
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