期刊
APPLIED PHYSICS LETTERS
卷 100, 期 7, 页码 -出版社
AMER INST PHYSICS
DOI: 10.1063/1.3684872
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资金
- A*STAR, Singapore [092 101 0055]
We present an efficient hybrid solar cell based on poly (3,4-ethylene-dioxythiophene): polystyrenesulfonate and planar Si with (100) and (111) orientations. The effect of Si surface native oxide on cell performance is studied. Compared to cell with hydrogen-terminated Si surface, the cell with oxygen-terminated Si surface reveals a 530-fold increase in power conversion efficiency (PCE) from 0.02% to 10.6%. The formation of SiOx-Si bonds poses a net positive surface dipole which leads to a favorable band alignment for charge separation. However, thicker oxide degrades cell performance due to higher series resistance. This study demonstrates the highest PCE reported to-date in this field. (C) 2012 American Institute of Physics. [doi:10.1063/1.3684872]
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