期刊
APPLIED PHYSICS LETTERS
卷 101, 期 21, 页码 -出版社
AMER INST PHYSICS
DOI: 10.1063/1.4767390
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资金
- Singapore Ministry of Education [RG63/10]
- Singapore National Research Foundation through the Competitive Research Programme (CRP) [NRF-CRP5-2009-04]
We present the wavelength dependent optical nonlinearities of two terpyridine-based Zn(II)-coordinated rigid linear polymers. It is found that the polymers exhibit large saturable absorption behavior under resonant excitation, while strong and tunable 2-photon absorption behaviors are observed in the biological window of 700-900 nm. Interestingly, Z-scan results reveal that, the polymers also exhibit large positive nonlinear refraction at 1300 nm in the solutions even with a low concentration, accompanied by small 3-photon absorption. Our results suggest that the polymers will be promising in various photonic applications, such as mode locking, 2-photon biological imaging, and all-optical switching. (C) 2012 American Institute of Physics. [http://dx.doi.org/10.1063/1.4767390]
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