期刊
APPLIED PHYSICS LETTERS
卷 99, 期 13, 页码 -出版社
AMER INST PHYSICS
DOI: 10.1063/1.3643044
关键词
circular dichroism; exchange interactions (electron); Fermi level; ferromagnetic materials; ground states; II-VI semiconductors; localised states; magnetic moments; magnetic thin films; manganese; nitrogen; paramagnetic materials; photoelectron spectra; semiconductor thin films; valence bands; zinc compounds
资金
- JSPS, Japan [S22224005]
- VINNOVA
- SSF
- Grants-in-Aid for Scientific Research [22224005] Funding Source: KAKEN
We have investigated the electronic structure of ZnO:Mn and ZnO:Mn,N thin films using x-ray magnetic circular dichroism (XMCD) and resonance-photoemission spectroscopy. From the Mn 2p -> 3d XMCD results, it is shown that, while XMCD signals only due to paramagnetic Mn(2+) ions were observed in ZnO:Mn, nonmagnetic, paramagnetic, and ferromagnetic Mn(2+) ions coexist in ZnO:Mn,N. XMCD signals of ZnO:Mn,N revealed that the localized Mn(2+) ground state and Mn(2+) state hybridized with ligand hole coexisted, implying p-d exchange coupling. In the valence-band spectra, spectral weight near the Fermi level was suppressed, suggesting that interaction between magnetic moments in ZnO:Mn,N has localized nature. (C) 2011 American Institute of Physics. [doi: 10.1063/1.3643044]
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