期刊
JOURNAL OF PHYSICS-CONDENSED MATTER
卷 17, 期 10, 页码 1735-1746出版社
IOP PUBLISHING LTD
DOI: 10.1088/0953-8984/17/10/028
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We give a theoretical treatment of the interaction of electronic excitations (excitions) in biomolecules and quantum dots with the surrounding polar solvent. Significant quantum decoherence occurs due to the interaction of the electric dipole moment of the solute with the fluctuating electric dipole moments of the individual molecules in the solvent. We introduce spin boson models which could be used to describe the effects. of decoherence on the quantum dynamics of biomolecules which undergo light-induced conformational change and on biomolecules or quantum dots which are coupled by Forster resonant energy transfer.
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