期刊
ORGANIC LETTERS
卷 7, 期 8, 页码 1661-1663出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol0504300
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资金
- NIGMS NIH HHS [GM31077] Funding Source: Medline
Three novel domino reaction processes have been discovered and developed that employ the regioselective and stereoselective [Rh(CO)(2)Cl](2)-catalyzed alkylations of allylic trifluoroacetates with alpha-substituted sodiomalonates followed by an intramolecular Pauson-Khand annulation, a [5 + 2] cycloaddition, or a cycloisomerization. A unique aspect of the methodology is that a single catalyst is used to effect sequential transformations simply by increasing the temperature for the second reaction.
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