期刊
APPLIED CATALYSIS B-ENVIRONMENTAL
卷 154, 期 -, 页码 177-182出版社
ELSEVIER
DOI: 10.1016/j.apcatb.2014.02.027
关键词
N-doped carbon; Methanol fuel cell; Chitosan; Sustability; Platinum
资金
- National Natural Science Foundation of China
- National High Technology Research and Development Program of China (863 Program) [2012AA053401, 2013AA051002]
- National Basic Research Program of China (973 Program) [2012CB215500, 2012CB932800]
- Science & Technology Research Programs of Jilin Province [20102204, 20100420]
The economical, green and sustainable preparation of functional carbon materials is of interest for energy storage and conversion technology. Herein, a functional N-doped carbon material (NC) was obtained from green biomass and cheap carbon black. The as-prepared NC enables the formation of highly-dispersed Pt nanocatalyst. Interestingly, compared to a state-of-the-art commercial Pt/C catalyst, the as-prepared Pt/NC catalyst shows a superior electrocatalytic performance with a 1.4-fold improvement in mass activity and a 1.5-fold enhancement in stability for methanol electrooxidation reaction. Thus, the green and earth-abundant biomass materials exhibit the promise in designing and producing functional carbon materials for high-performance electrochemical devices. (C) 2014 Elsevier B.V. All rights reserved.
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