期刊
APPLIED CATALYSIS B-ENVIRONMENTAL
卷 160, 期 -, 页码 614-620出版社
ELSEVIER
DOI: 10.1016/j.apcatb.2014.05.028
关键词
ZnIn2S4; In-situ photo-assisted deposition; H-2 evolution; MoS2 co-catalyst; Photocatalysis
资金
- National Natural Science Foundation of China [21173260, 51072221, 91233202]
- Ministry of Science and Technology of the People's Republic of China (973 Project) [2012CB932903, 2012CB932904]
- Chinese Academy of Sciences
A new MoS2/ZnIn2S4 photocatalyst system has been designed for H-2 evolution under visible light irradiation (lambda > 420 nm), which was obtained by hydrothermal method to afford floriated ZnIn2S4 microspheres, and MoS2 co-catalyst was subsequently loaded onto the ZnIn2S4 surface via a facile in-situ photo-assisted deposition process. The effects of hydrothermal temperature, the In/Zn molar ratios on the crystal structure, morphology, optical property as well as photocatalytic activity have been investigated in detail. Especially, the loading amount and deposition method of the MoS2 co-catalyst are found to dramatically influence the photocatalytic activity of H-2 evolution. Up to 8.047 mmol h(-1) g(-1) of H-2 evolution rate has been achieved, 28 times higher than that of untreated ZnIn2S4. This work provides a new synthetic way to increase the photocatalytic activity of MoS2/ZnIn(2)S4. (C) 2014 Elsevier B.V. All rights reserved.
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