期刊
APPLIED CATALYSIS B-ENVIRONMENTAL
卷 138, 期 -, 页码 1-8出版社
ELSEVIER
DOI: 10.1016/j.apcatb.2013.02.029
关键词
Mesoporous; Carbon-incorporated ZnO; Solvothermal synthesis; Adsorption; Photodecolorization
资金
- Natural Science Foundation of China [21171146]
- Zhejiang Provincial Natural Science Foundation of China [Y4110304]
- Anhui Provincial Natural Science Foundation [11040606M53]
Uniform hamburger-like mesoporous carbon-incorporated ZnO (MC-ZnO) nanoarchitectures were facilely prepared by a simple, economical and environmentally benign solvothermal method using ethylene glycol (EG) as solvent in the presence of glucose. The as-obtained samples possessed a high surface area of 104 m(2) g(-1) and narrow pore size distribution around 7.2 nm. The adsorption behavior of Congo red (CR) onto the products fitted well the Langmuir isotherm and the adsorption process followed the pseudo-second-order kinetic model. The maximum adsorption capacity of CR as 162 mg g(-1) was achieved by Langmuir equation, while only 18.8 mg g(-1) was found for by commercial ZnO nanoparticles. Furthermore, the as-prepared nanoarchitectures exhibited enhanced photocatalytic activity for the decolorization of photosensitized dyes (CR and rhodamine-B) under visible-light illumination. Therefore, the MC-ZnO nanoarchitectures developed in this work may be a promising potential material for wastewater treatment. (C) 2013 Elsevier B.V. All rights reserved.
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