期刊
PHYSICAL REVIEW B
卷 72, 期 3, 页码 -出版社
AMERICAN PHYSICAL SOC
DOI: 10.1103/PhysRevB.72.035448
关键词
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Orbital-specific femtosecond charge transfer dynamics between Fe(II)-tetraphenylporphyrin molecules and semimetallic molybdenum disulfide substrates is investigated using core-level resonant photoemission spectroscopy. The electronic coupling to the substrate and the efficiency of charge transport across the interface is found to be different for the individual molecular electronic subsystems. In particular, electrons excited at the phenyl substituents are transferred within 3-6 fs, while hopping from the porphyrin ring is slower than 30 fs.
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