期刊
JOURNAL OF NANOSCIENCE AND NANOTECHNOLOGY
卷 5, 期 7, 页码 1081-1087出版社
AMER SCIENTIFIC PUBLISHERS
DOI: 10.1166/jnn.2005.149
关键词
layer-by-layer assembly; nanoparticles; super-hydrophilicity; thin films; biocompatibility
类别
资金
- NIBIB NIH HHS [1R01 EB00739-01] Funding Source: Medline
Stable, super-hydrophilic (water contact angle approximate to 0 degrees) titanium dioxide nanoparticle thin films have been obtained on substrates with different initial wettability such as glass, poly(methyl methacrylate) and poly(dimethyl siloxane) using layer-by-layer nano-assembly method. Titanium dioxide nanoparticles were alternated with poly(styrene sulfonate) to form films of thickness ranging from 11 nm to 220 nm. The hydrophilicity of these thin films increases with increasing number of deposited PSS/TiO2 bilayers. It was found that 2, 5 and 20 layers were needed to form super-hydrophilic TiO2 coating on glass, PMMA and PDMS respectively. Oxygen plasma treatment of substrate surfaces enhanced the formation of homogeneous TiO2 films and accelerated the formation of hydrophilic layers. Super-hydrophilicity has been shown to be unique to PSS/TiO2 films as compared with other polyelectrolyte/nanoparticle layers, and UV irradiation may restore hydrophilicity even after months of storing of the samples. Biocompatibility of TiO2 nanoparticle films has been demonstrated by the successful cell culture of human dermal fibroblast.
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