Deep inelastic neutron scattering from orthorhombic ordered HCl: Short-time proton dynamics and anomalous neutron cross sections

Deep inelastic neutron scattering measurements from orthorhombic ordered HCl are presented and analyzed in order to clarify the problem of an anomalous deficit in the neutron-proton cross section found in previous experiments on various materials. A reliable model for the HCl short-time single-particle dynamics, including atomic vibrational anisotropies and deviations from the impulsive approximation, is set up. The model HCl response function is transformed into simulated time-of-flight spectra, taking carefully into account the effects of instrumental resolution and the filter absorption profile used for neutron energy analysis. Finally, the experimental values of the anomalous reduction factor for the neutron-proton cross section are extracted by comparing simulated and experimental data. Results show a 34% reduction of the H cross section, varying with the scattering angle in a range centered at 53 degrees. In addition, the same approximate procedure used in earlier studies is also employed, providing results in reasonable agreement with the more rigorous ones, and confirming the substantial reliability of the past work on this subject.