4.8 Article

Atomic-scale sources and mechanism of nanoscale electronic disorder in Bi2Sr2CaCu2O8+δ

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SCIENCE
卷 309, 期 5737, 页码 1048-1052

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AMER ASSOC ADVANCEMENT SCIENCE
DOI: 10.1126/science.1113095

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The randomness of dopant atom distributions in cuprate high-critical temperature superconductors has long been suspected to cause nanoscale electronic disorder. In the superconductor Bi2Sr2CaCu2O8+delta, we identified populations of atomic-scale impurity states whose spatial densities follow closely those of the oxygen dopant atoms. We found that the impurity-state locations are strongly correlated with all manifestations of the nanoscale electronic disorder. This disorder occurs via an unanticipated mechanism exhibiting high-energy spectral weight shifts, with associated strong superconducting coherence peak suppression but very weak scattering of low-energy quasi-particles.

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