期刊
JOURNAL OF PHYSICS B-ATOMIC MOLECULAR AND OPTICAL PHYSICS
卷 38, 期 17, 页码 L277-L284出版社
IOP PUBLISHING LTD
DOI: 10.1088/0953-4075/38/17/L01
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We have measured photoelectron angular distributions in the molecular frame (MF-PADs) for O 1s photoemission from CO2, using photoelectron-O+-CO+ coincidence momentum imaging. Results for the molecular axis at 0, 45 and 90 to the electric vector of the light are reported. The major features of the MF-PADs are fairly well reproduced by calculations employing a relaxed-core Hartree-Fock approach. Weak asymmetric features are seen through a plane perpendicular to the molecular axis and attributed to symmetry lowering by anti-symmetric stretching motion.
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