期刊
JOURNAL OF THE AMERICAN CHEMICAL SOCIETY
卷 127, 期 38, 页码 13305-13311出版社
AMER CHEMICAL SOC
DOI: 10.1021/ja0524898
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A new nucleophilic catalytic system comprised of dialkylaminopyridine-functionalized mesoporous silica nanosphere (DMAP-MSN) has been synthesized and characterized. We have demonstrated that this material is an efficient heterogeneous catalyst for Baylis-Hillman, acylation, and silylation reactions with good reactivity, product selectivity, and recyclability. We envision that this DMAP-functionalized mesoporous silica material can also serve as an effective heterogeneous catalyst for many other catalytic nucleophilic reactions.
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