期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 11, 期 24, 页码 7146-7153出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.200500253
关键词
cooperative effects; homogeneous catalysis; hydrogen bonds; P ligands; proton transfer
Inspired by the cooperativity displayed by metalloenzymes, bifunctional organometallic complexes featuring pendant basic functional groups are designed and evaluated as catalysts in reactions for which enzymes are not suited. Anti-Markovnikov hydration of terminal alkynes is the focus, as are hydrogen bonding and proton transfer facilitated by the pendant groups.
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