期刊
PURE AND APPLIED CHEMISTRY
卷 78, 期 2, 页码 231-239出版社
WALTER DE GRUYTER GMBH
DOI: 10.1351/pac200678020231
关键词
multicomponent; palladium; heterocycle; synthesis; cascade reactions
In recent years, new processes based on transition-metal-mediated intramolecular addition reaction of heteronucleophiles and stabilized carbon nucleophiles to unactivated alkenes and alkynes have been developed in our laboratory. In this article, we summarize a number of recent synthetic applications of these new processes. Emphasis is placed on the development of multicomponent reactions based on a Pd-mediated intramolecular cyclization coupled with a carbon-carbon bond-forming reaction. Applications of this methodology to the synthesis of natural lignans are also reported.
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