期刊
JOURNAL OF AEROSOL SCIENCE
卷 37, 期 5, 页码 555-576出版社
PERGAMON-ELSEVIER SCIENCE LTD
DOI: 10.1016/j.jaerosci.2005.04.010
关键词
nanoparticles; coagulation; nodal methods; direct numerical simulation; Navier-Stokes equations; mixing layers
Direct numerical simulation of a coagulating aerosol in a two-dimensional, incompressible, iso-thermal shear layer is performed. The evolution of the particle field is obtained by utilizing a nodal model to approximate the aerosol general dynamic equation (GDE). The GDE is written in discrete form as a population balance on each particle size and describes particle dynamics under the influence of various physical phenomena: convection, diffusion, and coagulation. The nodal approach is advantageous in that there are no a priori assumptions regarding the nature of the particle size distribution and therefore does not suffer from the severe constraints of other methodologies. This approach divides the particle size distribution into bins, for each of which a transport equation is obtained. A coagulation Damkohler number is defined to represent the ratio of the convective time scale to the coagulation time scale. Simulations are performed at a Reynolds number of 200 and coagulation Damkohler numbers of 1 and 10. The nanoparticle field is presented as a function of space, time and size. Results indicate that strong spatial variations in the particle concentrations develop in time and that these spatial gradients act to increase the geometric standard deviation of the particle size distribution. As the coagulation Damkohler number is increased, particle growth increases and particle size distributions wider than the self-preserving limit are predicted. The capture of the evolution of the particle field as a function of space, time and size suggests that the methodology is sufficiently general and robust to be useful in predicting the growth and dynamics in inhomogeneous, and possibly, turbulent flows. (C) 2005 Elsevier Ltd. All rights reserved.
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