期刊
JOURNAL OF PHYSICAL CHEMISTRY A
卷 110, 期 20, 页码 6387-6390出版社
AMER CHEMICAL SOC
DOI: 10.1021/jp061028l
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Infrared and electronic spectroscopy was applied to the benzene-ammonia cluster cation in the gas phase, and the observed spectra revealed the formation of a new C-N valence bond between the benzene and ammonia moieties, which has been predicted by the quantum chemical calculations ( Tachikawa, H. Phys. Chem. Chem. Phys. 2002, 4, 6018). This cluster cation is regarded as a model for the cyclohexadienyl type intermediate in nucleophilic substitution reactions.
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