期刊
ORGANIC LETTERS
卷 8, 期 15, 页码 3275-3278出版社
AMER CHEMICAL SOC
DOI: 10.1021/ol061137i
关键词
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资金
- NIGMS NIH HHS [R01 GM059384-20, GM 059384, R01 GM059384] Funding Source: Medline
A new strategy for the synthesis of (+/-)-aspidophytine has been developed and is based on a Rh(II)-catalyzed cyclization/dipolar cycloaddition sequence. The resulting [3+2]-cycloadduct undergoes an efficient Lewis acid mediated cascade that rapidly provides the complete skeleton of aspidophytine. The synthesis also features a mild decarbomethoxylation reaction.
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