期刊
ADVANCED SYNTHESIS & CATALYSIS
卷 348, 期 12-13, 页码 1711-1718出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/adsc.200606059
关键词
asymmetric aldol reactions; catalysis; ionic liquids; proline; supported synthesis
Ionic-liquid-anchored (2S,4R)-4-hydroxyproline 12 catalyzes direct asymmetric aldol reactions with comparable enantioselectivities in DMSO, and with superior enantioselectivities in neat acetone or 2-butanone, than (S)-proline (8) (up to 28% ee difference) itself. Furthermore, the supported catalyst 12 can be easily recycled and reused for at least four times without significant loss of yields and enantioselectivity.
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