期刊
JOURNAL OF PHYSICAL CHEMISTRY A
卷 110, 期 31, 页码 9743-9757出版社
AMER CHEMICAL SOC
DOI: 10.1021/jp062192b
关键词
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资金
- NIGMS NIH HHS [R01 GM071684-02, R01 GM071684-04, R01 GM071684-03, R01 GM071684, R01 GM071684-01] Funding Source: Medline
We use Shannon's definition of information to develop a theory to predict a photon-counting-based single-molecule experiment's ability to measure the desired property. We treat three phenomena that are commonly measured on single molecules: spectral fluctuations of a solvatochromic dye; assignment of the azimuthal dipole angle; determination of a distance by fluorescence resonant energy transfer using Forster's theory. We consider the effect of background and other imperfections on the measurement through the decrease in information.
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