Indirect impact of atmospheric aerosols in idealized simulations of convective-radiative quasi equilibrium

This paper discusses a cloud-resolving modeling study concerning the impact of warm-rain microphysics on convective-radiative quasi equilibrium with fixed surface characteristics and prescribed solar input, both mimicking the mean conditions on earth. Two limits of the concentration of cloud droplets, either 100 cm(-3) (referred to as pristine) or 1000 cm(-3) (referred to as polluted), are considered. In addition, three formulations of the effective radius of water droplets in diluted cloudy volumes are used, corresponding to the homogeneous, intermediate, and extremely inhomogeneous mixing scenarios. The assumed concentration of cloud droplets, together with the assumed mixing scenario, affects the local value of the effective radius of cloud droplets (the first indirect aerosol effect, also known as the Twomey effect) and the transfer of cloud water into drizzle and rain, which can affect the mean cloudiness and the hydrologic cycle (the second indirect effect). The convective-radiative quasi equilibrium mimics the estimates of globally and annually averaged water and energy fluxes across the earth's atmosphere to within less than 10 W m(-2). As on earth, the model cloudiness is dominated by shallow convection. It is found that the impact of warm microphysics is dominated by the first indirect effect, whereas the second indirect effect has a smaller impact. The assumed droplet concentration and mixing scenario impact the mean planetary albedo and, thus, the amount of solar energy reaching the surface, with all other components of atmospheric energy and water budgets virtually the same in all simulations. The weak second indirect effect highlights the difference between the impact of cloud microphysics on a single cloud and the impact on an ensemble of clouds, with only the latter including the feedbacks between clouds and their environment. The formulation of the effective radius in the diluted cloudy volumes turns out to be of critical importance, with the amount of solar energy reaching the surface being the same in the pristine case assuming the homogeneous mixing scenario and in the polluted case with the extremely inhomogeneous mixing. This result emphasizes the essential role of poorly understood microphysical transformations within diluted convective clouds, which strongly impact the magnitude of the first indirect (Twomey) effect. Implications for future research in this area are discussed.