期刊
JOURNAL OF CHEMICAL PHYSICS
卷 125, 期 22, 页码 -出版社
AMER INST PHYSICS
DOI: 10.1063/1.2397686
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资金
- NIGMS NIH HHS [2R01-GM59230-05] Funding Source: Medline
Polarization tuning of the interference of chirality-induced tensor components is used to simulate the suppression of diagonal peaks and amplification of cross peaks in femtosecond two-dimensional photon echo signals of excitons in a chiral porphyrin dimer. Superpositions of various tensor components which generate the optimized signals are constructed using a genetic learning algorithm. Exciton couplings and bath correlations may be extracted from these highly resolved signals. (c) 2006 American Institute of Physics.
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