期刊
CHEMISTRY-A EUROPEAN JOURNAL
卷 13, 期 24, 页码 6883-6890出版社
WILEY-V C H VERLAG GMBH
DOI: 10.1002/chem.200700501
关键词
cluster compounds; gas-phase reactions; heterogeneous catalysis; isotope scrambling; platinum
Rates for the dihydrogen elimination of methane, ethane, and propane with cationic platinum clusters, Pt-n(+) (1 <= n <= 21), were measured under binary collision conditions in a Fourier transform ion cyclotron resonance mass spectrometer (FTICR). The reaction rate for a given cluster, Pt-n(+), follows the trend k(CH4)
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